Browsing Atmospheric Sciences by Subject "Atmospheric chemistry"
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Analysis Of Model And Observation Data For The Development Of A Public Pm2.5 Air-Quality Advisories Tool (Aquat)An air-quality advisory tool (AQuAT) that combines mobile measurements of particulate matter less than or equal to 2.5mum in diameter (PM2.5) with air-quality simulations performed with the Alaska adapted version of the Community Multiscale Air Quality (CMAQ) model was developed to interpolate PM2.5-measurements into unmonitored neighborhoods in Fairbanks, Alaska. AQuAT was developed as traditional interpolation methods of interpolating the mobile measurements were unsuccessful. Such a spatially differentiated air-quality advisory is highly desired in Fairbanks due to health concerns of PM2.5, and the need to improve the quality of life. The accuracy of AQuAT depends on the accuracy of the air-quality simulations used for its database. Evaluation of these simulations showed that they captured the observed relationships between PM2.5-concentrations and major meteorological fields (e.g., wind-speed, temperature, and surface-inversions) well. Skill scores for simulated PM2.5-concentrations fell in the range of modern models. The AQuAT database can include information on the nonlinear impacts of various emission sources on PM2.5-concentrations. This benefit was illustrated by investigating the impacts of emissions from point sources, uncertified wood-burning devices, and traffic on the distribution of PM 2.5-concentrations in the neighborhoods. Sensitivity studies on the effects of wood-burning device changeouts on the PM2.5-concentrations suggested that the emission inventory should be updated as soon as possible to capture recent changes in the emission situation in response to the changeout program. The performance of AQuAT was evaluated with PM2.5-measurements from mobile and stationary sites, and with simulated PM2.5-concentrations of winter 2010/2011 which were assumed to be "grand-truth" data. These evaluations showed that AQuAT captured the magnitudes and temporal evolutions of the PM 2.5-measurements and the "grand-truth" data well. The inclusion of wind-speed, wind-direction, and temperature in AQuAT did not improve its accuracy. This result may be explained by the fact that the relationships between meteorology and PM2.5-concentrations were already captured by the database. AQuAT allows quick spatial interpolation after the mobile measurements were made and provides error bars. It also allows for any route within the area for which a database of simulated concentrations exists. It was shown that AQuAT can be easily transferred for applications in other regions.